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  • 1.
    Jacobs, Anna
    et al.
    STFI.
    Lundqvist, Jon
    Lund university, Sweden.
    Stålbrand, Henrik
    Lund university, Sweden.
    Tjerneld, Folke
    Lund university, Sweden.
    Dahlman, Olof
    STFI.
    Characterization of water-soluble hemicelluloses from spruce and aspen employing SEC/MALDI mass spectroscopy2002In: Carbohydrate Research, ISSN 0008-6215, E-ISSN 1873-426X, Vol. 337, no 8, p. 711-717Article in journal (Refereed)
  • 2.
    Jacobs, Anna
    et al.
    STFI.
    Palm, Magnus
    Lund university, Sweden.
    Zacchi, Guido
    Lund university, Sweden.
    Dahlman, Olof
    STFI.
    Isolation and characterization of water-soluble hemicelluloses from flax shive2003In: Carbohydrate Research, ISSN 0008-6215, E-ISSN 1873-426X, Vol. 338, no 18, p. 1869-1876Article in journal (Refereed)
  • 3.
    Lindh, Erik L.
    et al.
    RISE, Innventia. KTH Royal Institute of Technology, Sweden.
    Bergenstråhle-Wohlert, Malin
    RISE, Innventia. KTH Royal Institute of Technology, Sweden.
    Terenzi, Camilla
    KTH Royal Institute of Technology, Sweden.
    Salmen, Lennart
    RISE, Innventia. KTH Royal Institute of Technology, Sweden.
    Furo, István
    KTH Royal Institute of Technology, Sweden.
    Non-exchanging hydroxyl groups on the surface of cellulose fibrils: The role of interaction with water2016In: Carbohydrate Research, ISSN 0008-6215, E-ISSN 1873-426X, Vol. 434, p. 136-142Article in journal (Refereed)
    Abstract [en]

    The interaction of water with cellulose stages many unresolved questions. Here 2H MAS NMR and IR spectra recorded under carefully selected conditions in 1H-2H exchanged, and re-exchanged, cellulose samples are presented. It is shown here, by a quantitative and robust approach, that only two of the three available hydroxyl groups on the surface of cellulose fibrils are exchanging their hydrogen with the surrounding water molecules. This finding is additionally verified and explained by MD simulations which demonstrate that the 1HO(2) and 1HO(6) hydroxyl groups of the constituting glucose units act as hydrogen-bond donors to water, while the 1HO(3) groups behave exclusively as hydrogen-bond acceptors from water and donate hydrogen to their intra-chain neighbors O(5). We conclude that such a behavior makes the latter hydroxyl group unreactive to hydrogen exchange with water.

  • 4.
    Teleman, Anita
    et al.
    STFI.
    Nordström, Maria
    STFI.
    Tenkanen, Maija
    VTT, Finland.
    Jacobs, Anna
    STFI.
    Dahlman, Olof
    STFI.
    Isolation and characterization of O-acetylated glucomannans from aspen and birch wood2003In: Carbohydrate Research, ISSN 0008-6215, E-ISSN 1873-426X, Vol. 338, no 6, p. 525-534Article in journal (Refereed)
  • 5.
    Teleman, Anita
    et al.
    STFI.
    Tenkanen, Maija
    VTT, Finland.
    Jacobs, Anna
    STFI.
    Dahlman, Olof
    STFI.
    Characterization of O-acetyl-(4-O-methylglucurono)xylan isolated from birch and beech2002In: Carbohydrate Research, ISSN 0008-6215, E-ISSN 1873-426X, Vol. 337, no 4, p. 373-377Article in journal (Refereed)
1 - 5 of 5
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