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Stereoselective Catalytic Synthesis of Bioactive Compounds in Natural Deep Eutectic Solvents (NADESs): A Survey across the Catalytic Spectrum
University of Évora, Portugal.
RISE Research Institutes of Sweden, Bioeconomy and Health, Chemical Process and Pharmaceutical Development. University of Évora, Portugal; ChiraTecnics, Portugal.ORCID iD: 0000-0001-5781-1689
University of Évora, Portugal; ChiraTecnics, Portugal.
University of Évora, Portugal; Universidade de Coimbra, Portugal; .
2024 (English)In: Catalysts, E-ISSN 2073-4344, Vol. 14, no 3, article id 160Article in journal (Refereed) Published
Abstract [en]

Deep eutectic solvents (DESs) are a mixture of two or more components, and at a particular composition, they become liquids at room temperature. When the compounds that constitute the DESs are primary metabolites namely, amino acids, organic acids, sugars, or choline derivatives, the DESs are called natural deep eutectic solvents (NADESs). NADESs fully represent green chemistry principles. These solvents are highly welcome, as they are obtained from renewable resources, and gratifyingly are biodegradable and biocompatible. They are an alternative to room-temperature ionic liquids (RTILs). From the pharmaceutical industry’s point of view, they are highly desirable, but they unfortunately have been rarely used despite their enormous potential. In this review, we look at their impact on the asymmetric catalytic synthesis of key target molecules via metal-based catalysis, biocatalysis, and organocatalysis. In many cases, the NADESs that have been used are chiral and can even promote enantioselective reactions; this crucial and very exciting aspect is also discussed and analyzed. © 2024 by the authors.

Place, publisher, year, edition, pages
Multidisciplinary Digital Publishing Institute (MDPI) , 2024. Vol. 14, no 3, article id 160
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Chemical Sciences
Identifiers
URN: urn:nbn:se:ri:diva-72833DOI: 10.3390/catal14030160Scopus ID: 2-s2.0-85188683010OAI: oai:DiVA.org:ri-72833DiVA, id: diva2:1857803
Note

EPC acknowledges the Fundação para a Ciência e a Tecnologia (FCT) for funding through the strategic project to LAQV-REQUIMTE (FCT/MCTES; UIDB/50006/2020|UIDP/50006/2020). AJB acknowledges FCT for funding through the strategic project UIDB/00313/2020|UIDP/00313/2020 to Coimbra Chemistry Centre—Institute of Molecular Sciences (CQC-IMS)

Available from: 2024-05-14 Created: 2024-05-14 Last updated: 2024-05-14Bibliographically approved

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Federsel, Hans-Jürgen

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