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Formation and Out-of-Equilibrium, High/Low State Switching of a Nitroaldol Dynamer in Neutral Aqueous Media
KTH Royal Institute of Technology, Sweden.
KTH Royal Institute of Technology, Sweden.
KTH Royal Institute of Technology, Sweden.
RISE Research Institutes of Sweden, Bioekonomi och hälsa, Kemiska processer och läkemedel.ORCID-id: 0000-0002-3350-0242
Vise andre og tillknytning
2020 (engelsk)Inngår i: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 59, nr 9, s. 3434-3438Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

The nitroaldol reaction is demonstrated as an efficient dynamic covalent reaction in phosphate buffers at neutral pH. Rapid equilibration was recorded with pyridine-based aldehydes, and dynamic oligomerization could be achieved, leading to nitroaldol dynamers of up to 17 repeating units. The dynamers were applied in a coherent stimuli-responsive molecular system in which larger dynamers transiently existed out-of-equilibrium in a neutral aqueous system rich in formaldehyde, controlled by nitromethane.

sted, utgiver, år, opplag, sider
Wiley-VCH Verlag , 2020. Vol. 59, nr 9, s. 3434-3438
Emneord [en]
dynamers, formaldehyde, nitroaldol, stimuli response, systems chemistry, Chemical engineering, Chemical reactions, Chemistry, Covalent reaction, Molecular systems, Out of equilibrium, Phosphate buffers, Stimuli-responsive
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Identifikatorer
URN: urn:nbn:se:ri:diva-43973DOI: 10.1002/anie.201911706Scopus ID: 2-s2.0-85078789872OAI: oai:DiVA.org:ri-43973DiVA, id: diva2:1393852
Tilgjengelig fra: 2020-02-17 Laget: 2020-02-17 Sist oppdatert: 2023-12-07bibliografisk kontrollert

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