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2021 (English) In: Energy & Fuels, ISSN 0887-0624, E-ISSN 1520-5029, Vol. 35, no 23, p. 19705-Article in journal (Refereed) Published
Abstract [en] An innovative and simple method based on dilution, named as the dilution chamber (DC), allowing the measurement of solid and condensable fractions of particulate matter emitted by residential wood combustion appliances has been developed, and its performances have been evaluated. The DC method was then tested by five European institutes (Ineris, ISSI/ENEA, DTI, and RISE) on advanced residential wood log/pellet stoves, under nominal output and low output combustion conditions and using different fuel types. The aim of the study was to evaluate the capability of the DC method to collect the condensable fraction. The DC method was compared with another manual method used to collect the solid and condensable fractions at the same time, the dilution tunnel (DT), on four sampling platforms. A third method, a combining heated filter and impinger filled in with isopropanol collection (SPC-IPA), was also used by Ineris only for comparison with the DC method. PM measurements based on the DC method globally showed a linear correlation with PM measurements based on DT (R2 ranged between 0.81 and 0.99, p < 0.05) specifically for the residential wood stoves under low output conditions when the condensable fraction contributes the most. An analysis and quantification of PAHs related to the total mass of PM of samples taken by the DC method and performed by ENEA/ISSI showed that it produces a condensation effect of semivolatile species comparable or even greater than the DT method. PM emission factors calculated from PM measurements based on the DC method were (i) about 2- to 20-fold higher for the residential wood stoves (EF ranged between 201 to 2420 g GJ-1) compared to those obtained for the residential pellet stoves (EF ranged between 108 to 556 g GJ-1) and (ii) of the same magnitude of PM emission factors from the literature or the EMEP/EEA air pollutant emission inventory guidebook.
Place, publisher, year, edition, pages
American Chemical Society, 2021
Keywords Combustion, Dilution, Stoves, Wood, Emission factors, Innovative method, Measurement-based, Measurements of, Particulate Matter, Performance, PM emissions, Residential wood combustions, SIMPLE method, Wood stove, Housing
National Category
Energy Engineering
Identifiers urn:nbn:se:ri:diva-57367 (URN) 10.1021/acs.energyfuels.1c02595 (DOI) 2-s2.0-85119917131 (Scopus ID)
Note Funding details: Horizon 2020 Framework Programme, H2020; Funding details: European Metrology Programme for Innovation and Research, EMPIR; Funding details: National Physical Laboratory, NPL; Funding text 1: This work has been supported by the European Metrology Program for Innovation and Research (EMPIR) in the project context IMPRESS 2 coordinated by NPL UK. The EMPIR initiative is cofunded by the European Union’s Horizon 2020 research and innovation program and the EMPIR Participating States. Financial support from H2020 program is gratefully acknowledged. We thank all participants of the IMPRESS 2 project: the coordinator (NPL) and all the other National Metrology Institutes (CEM, CMI, PTB, RISE, VSL, VTT, CNR, DTI, DTU, ISSI, ENEA, Ineris, TU Delft, and UC3M). Ineris thanks Nicolas Karoski, Adrien Dermigny, Mehdi Dionigi, and Lars Schwarzer for their contribution to the combustion tests.
2021-12-172021-12-172023-06-07 Bibliographically approved